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05. Heero Yuy and Duo Maxwell (Gundam Wing)
Either you believe they're straight, gay or bi...you have to admit there is a certain something about the two. Some "chemicals between them". There's a certain believable aspect to the idea of the overly talkative Duo winning over the quiet and jaded Heero's heart.
04. Rogue and Gambit (X-Men)
Ever since I was little and was first introduced to X-men I've been obsessed with this couple. I watched the cartoons and, for me, the couple was advanced when I could see and hear the two actually talk to one another in their cute accents. Both passionate, but plagued with Rogue's powers (not being able to be touched without sucking the energy from the touchee). Sorta like star-crossed lovers in a way. ^_^;;
03. Spike and Drusilla (Buffy the Vampire Slayer)
I can't say I'm much of a Buffy fan anymore, I haven't watched it in about 2 or 3 seasons... But I remember the season with Spike and Dru and that one season was my favorite. The two were sexy, dark and so completely in love. It's the sort of relationship all dark goth girls dream of, a fantasy come true. Watching the twisted and not-quite-there Dru be spoiled by the cruel and intense Spike was more enjoyable than watching the somewhat mushy Buffy and Angel most of the time.
02. Pirotes and Ashram (Record of Lodoss War)
Pirotes and Ashram are both so like one another it was crazy. Both were so devoted to a cause, Ashram to the war at hand, Pirotes to her love for Ashram. One of the best scenes between a couple I'd ever seen was when Pirotes sliced her arm with a dagger and declared to Ashram she would return to him before it healed. If that's not ramance, I don't know what is.
01. Harley Quinn and the Joker (Batman)
I love Batman to begin with and in the series when they introduce Harley Quinn I was amazed. The two are totally nuts, but they are the most amusing couple ever to be conceived. I have a thing for bad guys if you haven't noticed... They just are so happy together, smiling after they blow something up with their devlish smiles. It's actually sorta cute.
Others I considered...
Kusanagi and Momiji (Blue Seed)
Lina Inverse and Gourry Gabriev (Slayers)
Rinoa & Squall (Final Fantasy 8)
Sohma Kyou and Honda Tohru (Fruits Basket)
Heero Yuy and Duo Maxwell (Gundam Wing)
Heero Yuy and Relena Peacecraft (Gundam Wing)